Plasmon-Enhanced MoS2 Photodetector Enabled by Lithographically Patterned Au Disk Arrays and an h-BN Tunneling Layer
DOI:
https://doi.org/10.6919/ICJE.202603_12(3).0011Keywords:
MoS2; Plasmonics; Photodetector; Hot electrons.Abstract
High-performance visible light photodetection holds significant application value in optical communications, imaging, and sensing. Here, we demonstrate a plasmon-enhanced photodetector based on few-layer MoS2 integrated with Au disk arrays fabricated by direct writing lithography and a monolayer h-BN tunneling layer. The Au disk arrays (diameter: 1.5 μm, period: 2.5 μm, thickness: 40 nm), fabricated by direct writing lithography,offer excellent scalability and position controllability. The monolayer h-BN serves as a tunneling layer that not only prevents direct contact between Au and MoS2, suppressing dark current and photoluminescence quenching, but also enables the tunneling of plasmon-generated hot electrons into MoS2. Benefiting from the synergistic effects of near-field optical enhancement, hot electron tunneling injection, and strain-induced band modulation, the device exhibits significantly improved photoelectric conversion efficiency. Under 635 nm illumination at an ultralow power density of 0.01 mW/cm2, the device achieves a responsivity of 1384 A/W and a detectivity of 9.73 × 1013 Jones, along with stable and fast photoswitching response featuring rise/fall times of 40 ms/138 ms. Finite-difference time-domain simulations confirm pronounced electric field enhancement at the MoS2 layer induced by the Au disk arrays. This work provides a feasible design strategy for high-performance and scalable two-dimensional material photodetectors.
Downloads
References
[1] A. Elbanna, H. Jiang, Q. Fu, et al., 2D Material Infrared Photonics and Plasmonics. ACS Nano, 2023. 17(5): p. 4134–4179.
[2] C. Wang, Q. Wu, Y. Ding, et al., High-Responsivity and Broadband MoS2 Photodetector Using Interfacial Engineering. ACS Applied Materials & Interfaces, 2023. 15(39): p. 46236–46246.
[3] X. Li, J. ZhuB. Wei, Hybrid nanostructures of metal/two-dimensional nanomaterials for plasmon-enhanced applications. Chemical Society Reviews, 2016. 45(11): p. 3145–3187.
[4] J. An, X. Zhao, Y. Zhang, et al., Perspectives of 2D Materials for Optoelectronic Integration. Advanced Functional Materials, 2022. 32(14).
[5] J. Zha, M. Luo, M. Ye, et al., Infrared Photodetectors Based on 2D Materials and Nanophotonics. Advanced Functional Materials, 2022. 32(15).
[6] N. Goel, A. Kushwaha, S. Agarwal, et al., A critical review of recent advances, prospects, and challenges of MoS2/Si heterostructure based photodetectors. Journal of Alloys and Compounds, 2025. 1010.
[7] Y. Wang, G. Zhou, Z. Zhang, et al., Graphene-, Transition Metal Dichalcogenide-, and MXenes Material-Based Flexible Optoelectronic Devices. Nanomaterials, 2025. 16(1).
[8] W. Wang, X. Zeng, J. Warner, et al., Photoresponse-Bias Modulation of a High-Performance MoS2 Photodetector with a Unique Vertically Stacked 2H-MoS2/1T@2H-MoS2 Structure. ACS Applied Materials & Interfaces, 2020. 12(29): p. 33325–33335.
[9] X. Xu, R. Duan, W. Qi, et al., Manipulating Carrier Behavior by the Size Effect of Decoration in MoS2 Photodetectors. Advanced Optical Materials, 2025. 13(6).
[10] O. Yi, C. Zhang, J. Wang, et al., Gate-Tunable Dual-Mode Optoelectronic Device for Self-Powered Photodetector and Optoelectronic Synapse. Advanced Science, 2025. 12(17).
[11] J. Zou, Y. Huang, W. Wang, et al., Plasmonic MXene Nanoparticle-Enabled High-Performance Two-Dimensional MoS2 Photodetectors. ACS Applied Materials & Interfaces, 2022. 14(6): p. 8243–8250.
[12] P. Vashishtha, I. Abidi, S. Giridhar, et al., CVD-Grown Monolayer MoS2 and GaN Thin Film Heterostructure for a Self-Powered and Bidirectional Photodetector with an Extended Active Spectrum. ACS Applied Materials & Interfaces, 2024. 16(24): p. 31294–31303.
[13] C. YanH. Liu, Multifunctional Phototransistor Based on MoS2/Ta2NiSe5/WSe2 vdW Heterojunctions with High-Performance Anti-Ambipolar Transport. Advanced Optical Materials, 2026. 14(4).
[14] K. Ponnusamy, J. Bong, H. Lee, et al., Promoter-Free Synthesis of Wafer-Scale Monolayer MoS2 for Visible to Near-Infrared Photodetection. ACS Applied Materials & Interfaces, 2026. 18(1): p. 1995–2008.
[15] W. WangL. Qi, Light Management with Patterned Micro- and Nanostructure Arrays for Photocatalysis, Photovoltaics, and Optoelectronic and Optical Devices. Advanced Functional Materials, 2019. 29(25).
[16] J. Miao, W. Hu, Y. Jing, et al., Surface Plasmon-Enhanced Photodetection in Few Layer MoS2 Phototransistors with Au Nanostructure Arrays. Small, 2015. 11(20): p. 2392–2398.
[17] J. Guo, S. Li, Z. He, et al., Near-infrared photodetector based on few-layer MoS2 with sensitivity enhanced by localized surface plasmon resonance. Applied Surface Science, 2019. 483: p. 1037–1043.
[18] S. Ghopry, S. Alzahrani, B. Liu, et al., Dimensionally controlled MoS2 nanodiscs for optimal localized surface plasmonic resonance in nanohybrid photodetectors. Nano Express, 2025. 6(4).
[19] Y. Liu, R. Cheng, L. Liao, et al., Plasmon resonance enhanced multicolour photodetection by graphene. Nature Communications, 2011. 2.
[20] R. Xing, X. Zhang, X. Fan, et al., Coupling Strategies of Multi-Physical Fields in 2D Materials-Based Photodetectors. Advanced Materials, 2025. 37(16).
[21] L. Liu, Y. Guo, H. Shang, et al., Visible-Blind Spectrally Selective Near-Infrared Photodetection with Enhanced Sensitivity. ACS Applied Materials & Interfaces, 2025. 17(49): p. 66956–66964.
[22] T. Fayad, M. Eisa, E. Salih, et al., Self-biased visible-NIR photodetection enabled via a dual-heterojunction n-MoS2/p-CuO/n-Si design. Materials Advances, 2026. 7(2): p. 1265–1271.
[23] Y. Huang, C. Chen, C. Huang, et al., Flexible 2D material hetero-structure photodetectors with high responsivities, tunable wavelengths and short response times. 2D Materials, 2026. 13(1).
[24] D. Sahu, S. DasS. Ray, Plasmonic Au/MoxW1-xS2/Si Heterojunction for Broadband Photodetection. ACS Applied Materials & Interfaces, 2026. 18(1): p. 2109–2121.
[25] Z. Peng, X. Chen, Y. Fan, et al., Strain engineering of 2D semiconductors and graphene: from strain fields to band-structure tuning and photonic applications. Light: Science & Applications, 2020. 9(1).
[26] D. Lu, Y. Chen, L. Kong, et al., Strain-Plasmonic Coupled Broadband Photodetector Based on Monolayer MoS2. Small, 2022. 18(14).
[27] X. Hu, J. Li, H. Ji, et al., Achieving dark current suppression and photocurrent enhancement simultaneously in 2D MoS2 photodetector via Ag nanocluster modification. Nano Research, 2026. 19(1).
[28] X. Zhou, Z. Weng, J. Li, et al., Enhanced Photoelectric Response in MoS2/Graphene Heterostructures via Surface Plasmon Resonance. ACS Applied Nano Materials, 2026. 9(2): p. 1195–1204.
[29] H. Dong, Q. Yin, Z. Wu, et al., Visible-near infrared broadband photodetector enabled by a photolithography-defined plasmonic disk array. Photonics Research, 2025. 13(2): p. 453–467.
[30] M. Zhang, G. Zeng, G. Wu, et al., Van der Waals integrated plasmonic Au array for self-powered MoS2 photodetector. Applied Physics Letters, 2023. 122(25).
[31] H. Wang, Z. Li, D. Li, et al., Van der Waals Integration Based on Two-Dimensional Materials for High-Performance Infrared Photodetectors. Advanced Functional Materials, 2021. 31(30).
[32] S. Roy, S. Aktar, A. Tamang, et al., 0D/2D Nanomaterials Heterostructures for High-Performance Photodetectors: Combining Quantum Dots With 2D Materials. Small, 2026.
[33] J. He, Y. Yang, Y. He, et al., Low Noise and Fast Photoresponse of Few-Layered MoS2 Passivated by MA3Bi2Br9.ACS Photonics, 2018. 5(5): p. 1877–1884.
[34] Q. Zhang, B. Zhao, J. Chen, et al., High-Speed, High-Responsivity on-Chip Monolayer MoS2 Photodetector at Telecom Wavelengths. ACS Photonics, 2026. 13(4): p. 913–919.
Downloads
Published
Issue
Section
License
Copyright (c) 2026 International Core Journal of Engineering

This work is licensed under a Creative Commons Attribution-NonCommercial 4.0 International License.




